Unfortunately for you, Light Fingers is the only Ambition to still not have received any updates. The other three have received one each, with one to go.
Have you done the Wars of Illusion story? It used to be pretty hard to find, though that’s changed now due to trackers (see below). There’s also the Mind of a Long-Dead God, accessible from London with Stormy-Eyed 19. The only way to get that quality so high is by spending a while on Mutton Island, Bidding the Wind Speak when Time Passing in the Southern Archipelago is under 7.
About a year ago, quality trackers were introduced to streamline and better organize major stories for the four main stats. At the time, all existing users were thrown into MUST storylets (the ones you can’t back out of) allowing them to keep their progress or reset some of the stories* to replay the content. I don’t know if this event is still around, but if you haven’t gotten it and would like to see the changes you could contact Failbetter at support@failbettergames.com for assistance. The four tracking qualities are A Name in Seven Secret Alphabets for Watchful, A Name Whispered in Darkness for Shadowy, A Name Scrawled in Blood for Dangerous, and A Name Signed with a Flourish for Persuasive.
*The exceptions being players who completed the University storyline could not reset any of the Watchful content, and players exiled from Court could not reset any Persuasive content. Rare items were provided as compensation.
You also mentioned you’d like to become an Exceptional Friend again, for which things have changed slightly. In addition to House of Chimes access and the action/card perks, Exceptional Friends now get a special story once a month. Specifically, Exceptional Friends can begin the current Exceptional Story at any point in the month, the story changing over on the last Thursday of the month*. (After doing the global intro storylet visible to everyone and the first event in the House of Chimes**, each story can be completed at leisure even if you end your Exceptional Friendship.) Exceptional Stories began in May 2015 for a total of 17 so far; past ESes can be purchased on the Fate page for a higher price, several months after they were available to EFs. A more recent addition is Exceptional Seasons, in which completing the three consecutive stories unlocks a small bonus story; so far the seasons have been Heart’s Blood, Family Ties, Revolution, and the in-progress Wrecks.
*As such, one month’s purchase of Exceptional Friendship will typically allow access to two of the monthly stories, and occasionally with precise timing gives three.
**The current season is structured a little differently, so the stories are unlocked through the globally-accessed Breakwater House location instead of the House of Chimes.